Supercontinuum

In optics, a supercontinuum is formed when a collection of nonlinear processes act together upon a pump beam in order to cause severe spectral broadening of the original pump beam, for example using a microstructured optical fiber. The result is a smooth spectral continuum (see figure 1 for a typical example). There is no consensus on how much broadening constitutes a supercontinuum; however researchers have published work claiming as little as 60 nm of broadening as a supercontinuum. There is also no agreement on the spectral flatness required to define the bandwidth of the source, with authors using anything from 5 dB to 40 dB or more. In addition the term supercontinuum itself did not gain widespread acceptance until this century, with many authors using alternative phrases to describe their continua during the 1970s, 1980s and 1990s. In optics, a supercontinuum is formed when a collection of nonlinear processes act together upon a pump beam in order to cause severe spectral broadening of the original pump beam, for example using a microstructured optical fiber. The result is a smooth spectral continuum (see figure 1 for a typical example). There is no consensus on how much broadening constitutes a supercontinuum; however researchers have published work claiming as little as 60 nm of broadening as a supercontinuum. There is also no agreement on the spectral flatness required to define the bandwidth of the source, with authors using anything from 5 dB to 40 dB or more. In addition the term supercontinuum itself did not gain widespread acceptance until this century, with many authors using alternative phrases to describe their continua during the 1970s, 1980s and 1990s. During the last decade, the development of supercontinua sources has emerged as a research field. This is largely due to new technological developments, which have allowed more controlled and accessible generation of supercontinua. This renewed research has created a variety of new light sources which are finding applications in a diverse range of fields, including optical coherence tomography, frequency metrology, fluorescence lifetime imaging, optical communications, gas sensing and many others. The application of these sources has created a feedback loop whereby the scientists utilising the supercontinua are demanding better customisable continua to suit their particular applications. This has driven researchers to develop novel methods to produce these continua and to develop theories to understand their formation and aid future development. As a result, rapid progress has been made in developing these sources since 2000. While supercontinuum generation has for long been the preserve of fibers, in recent years, integrated waveguides have come of age to produce extremely broad spectra, opening the door to more economical, compact, robust, scalable and mass-producible supercontinuum sources. In 1964 Jones and Stoicheff reported using a continua generated by a maser to study induced Raman absorption in liquids at optical frequencies. It had been noted by Stoicheff in an early publication that 'when the maser emission was in a single sharp spectral line, all the Raman emission lines were sharp; whenever the maser emission contained additional components, all of the Raman emission lines, with the exception of the first Stokes line, were considerably broadened, sometimes up to several hundred cm−1.' These weak continua, as they were described, allowed the first Raman absorption spectroscopy measurements to be made. In 1970 Alfano and Shapiro reported the first measurements of frequency broadening in crystals and glasses using a frequency doubled Nd:Glass mode-locked laser. The output pulses were approximately 4 ps and had a pulse energy of 5 mJ. The filaments formed produced the first white light spectra in the range from 400-700 nm and the authors explained their formation through self-phase modulation and four-wave mixing. The filaments themselves were of no real use as a source; nevertheless the authors suggested that the crystals might prove useful as ultrafast light gates. Alfano is the discoverer and inventor of the supercontinuum in 1970 with three seminal articles in same issue of Phy Rev Letters (24, 592,584,1217(1970)) on ultimate white light source now called supercontinuum. The study of atomic vapours, organic vapours and liquids by Raman absorption spectroscopy through the 1960s and 1970s drove the development of continua sources. By the early 1970s, continua formed by nanosecond duration flash lamps and laser-triggered breakdown spark in gases, along with laser excited fluorescence continua from scintillator dyes, were being used to study the excited states. These sources all had problems; what was required was a source that produced broad continua at high power levels with a reasonable efficiency. In 1976 Lin and Stolen reported a new nanosecond source that produced continua with a bandwidth of 110-180 nm centred on 530 nm at output powers of around a kW. The system used a 10-20 kW dye laser producing 10 ns pulses with 15-20 nm of bandwidth to pump a 19.5 m long, 7 μm core diameter silica fibre . They could only manage a coupling efficiency in the region of 5-10%. By 1978 Lin and Nguyen reported several continua, most notably one stretching from 0.7-1.6 μm using a 315 m long GeO 2 {displaystyle extstyle _{2}} doped silica fibre with a 33 μm core. The optical setup was similar to Lin's previous work with Stolen, except in this instance the pump source was a 150 kW, 20 ns, Q-switched Nd:YAG laser. Indeed, they had so much power available to them that two thirds was attenuated away to prevent damage to the fibre. The 50 kW coupled into the fibre emerged as a 12 kW continuum . Stokes lines were clearly visible up to 1.3 μm, at which point the continuum began to smooth out, except for a large loss due to water absorption at 1.38 μm. As they increased the launch power beyond 50 kW they noted that the continuum extends down into the green part of the visible spectrum. However, the higher power levels quickly damaged their fibre. In the same paper they also pumped a single mode fibre with a 6 μm core diameter and 'a few 100 m in length.' It generated a similar continuum spanning from 0.9 μm to 1.7 μm with reduced launch and output powers. Without realising it, they had also generated optical solitons for the first time. In 1980 Fujii et al. repeated Lin's 1978 setup with a mode-locked Nd:YAG. The peak power of the pulses was reported as being greater than 100 kW and they achieved better than 70% coupling efficiency into a 10 μm core single-mode Ge doped fibre. Unusually, they did not report their pulse duration. Their spectrum spanned the entire spectral window in silica from 300 nm to 2100 nm. The authors concerned themselves with the visible side of the spectrum and identified the main mechanism for generation to be four-wave mixing of the pump and Raman generated Stokes. However, there were some higher order modes, which were attributed to sum-frequency generation between the pump and Stokes lines. The phase-matching condition was met by coupling of the up-converted light and the quasi-continuum of cladding modes. A further advance was reported by Washio et al. in 1980 when they pumped 150 m of single-mode fibre with a 1.34 μm Q-switched Nd:YAG laser. This was just inside the anomalous dispersion regime for their fibre. The result was a continua which stretched from 1.15 to 1.6 μm and showed no discrete Stokes lines. Up to this point no one had really provided a suitable explanation why the continuum smoothed out between the Stokes lines at longer wavelengths in fibres. In the majority of cases this is explained by soliton mechanisms; however, solitons were not reported in fibres until 1985. It was realised that self-phase modulation could not account for the broad continua seen, but for the most part little else was offered as an explanation.