Measurement of polariton-polariton interaction strength in the Thomas-Fermi regime of polariton condensation

A bosonic condensate of exciton polaritons (light-matter quasiparticles in a semiconductor) is a paradigmatic non-equilibrium quantum system with a spontaneously established macroscopic coherence. Driven by an off-resonant pumping laser, the condensate coexists and interacts with an optically injected incoherent reservoir, rendering it difficult to separate polariton-polariton interactions from polariton-reservoir interactions. This issue undermines measurements of the key parameter of the system - the polariton-polariton interaction strength, with the reported values spread over a range of four orders of magnitude. Here, for the first time to our knowledge, we create an optically trapped exciton-polariton condensate in the Thomas-Fermi regime dominated by polariton-polariton interactions. This allows us to perform the most straightforward measurement of the interaction strength, resulting in values that agree well with theory. Our work serves to reduce the uncertainty regarding the strength of polariton-polariton interactions and offers a textbook "condensate in a box" platform for fundamental studies of interaction-driven effects.