Bell correlations between light and vibrations in diamond at ambient conditions

In this talk we show how time-resolved Raman spectroscopy can be combined with Time Correlated Single Photon Counting (TCSPC) to create and evidence entanglement between light and a collective molecular vibration (i.e. an optical phonon) [3]. We further show that the correlations are strong enough to violate the Bell Inequality, which provides the most stringent test for entanglement. We measure the decay of these hybrid photon-phonon Bell correlations with sub-picosecond time-resolution and find that they survive over several hundred oscillations at ambient conditions.