Superconducting order from local disorder
2020
In all Fe superconductors the maximal $T_c$ correlates with the average anion height above the Fe plane, i.e. with the geometry of the FeAs$_4$ or FeCh$_4$ (Ch = Te, Se, S) tetrahedron. By synthesizing FeSe$_{1-x}$S$_x$ (0 $\leq$ x $\leq$ 1) single crystal alloys and by performing a series of experiments we find that $T_c$ does scale with the average anion height for $x$ in the presence of nematic order and near FeS, whereas superconductivity changes for all other $x$ track local crystallographic disorder and disorder-related scattering. Our findings demonstrate the strong coupling between disorder and $T_c$ as $x$ is tuned beyond the nematic critical point (NCP) and provide evidence of a $T_c$ tuning mechanism related to local bond disorder.
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