Giant nonlinear electron-lattice interaction in cuprate superconductors, and origin of the pseudogap
2009
The pseudogap is a key property of the cuprate superconductors, whose understanding should illuminate the pairing mechanism. Recent experimental data support a close connection between the pseudogap and an oxygen-driven C4 symmetry breaking within the CuO2 plane unit cell. Using ab initio Molecular Dynamics, we demonstrate the existence of a strong nonlinear electron-oxygen vibrator coupling in two cuprates. In a mean field approach applied to this coupling within a model Hamiltonian, we derive a C4 splitting/pseudogap phase diagram in agreement with experiment - providing an explanation for the pseudogap phenomenon from first principles. The implications for superconductivity and the Fermi surface arc effect are discussed.
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