Regional and Global CO and Aerosol Correlations: An Integrated Approach of Surface, Satellite, and Aircraft Measurements and Model Simulations

We investigate regional and global CO and fine mode aerosol correlations by combining GOCART model simulations with various measurements from surface (CMDL /CO and AERONET / aerosol), satellite (MOPl3T / CO and MODIS / aerosol), and aircraft. CO mixing ratios and aerosol concentrations are examined using surface and aircraft measurements on several representative regions. Satellite observations provide the comparisons of CO column and aerosol fine model AOD at global scale. Numerical model simulation allows us to compare CO and aerosol properties without temporal and spatial limitation and with the capability to trace emissions by isolating different somces. Our zonal mean comparisons confirm the previous researches that the variations of CO and aerosol properties are out of phase by several month. over northern hemisphere middle latitudes where anthropogenic emissions dominate. Over the biomass burning dominating regions, such as southern hemisphere (SH) extra-tropical zone, the concentration and column properties of CO and aerosol show more agreement. Long- term transport and local chemistry drive the biggest phase shift of CO and aerosol properties over remote SH ocean regions. There are much more complicated relationships CO and aerosol properties over stations and small regions due to emission, transport, and local chemistry.