Observation of new particle formation in subtropical urban environment
2010
The aim of this study was to characterise the new particle formation events in subtropical
urban environment Southern Hemisphere. The study measured the number
concentration of particles and its size distribution in Brisbane, Australia during 2009.
The variation of particle number concentration and nucleation burst events were studied
and the particle growth rate was characterised which was first reported in urban
environment of Australia. The annual average NUFP, NAitken and Nnuc were 9.3×103,
3.7×103 and 5.6×103 cm−3, respectively. Weak seasonal variation in number concentration
was observed. Local vehicle emission was major contributor of the pollution
observed in the morning which was dominated by the Aitken mode particles, while particle
formed by secondary formation process was contributed to the particle number
concentration in the afternoon. 65 nucleation burst events were identified during the
study period. Nucleation burst events were classified into two groups with and without
particle growth after the burst of nucleation mode particles observed. Average particle growth rate of the nucleation events was 4.6 nmhr−1 (ranged from 1.79–7.78 nmhr−1).
Case studies of the nucleation burst events were characterised including i) the nucleation
burst with particle growth which was associated with the particle precursor emitted
from local vehicle emission, ii) the nucleation burst without particle growth which
was due to the transport of industrial emissions from the coast to Brisbane city, and iii)
interplay between the above two cases which demonstrated the impact of the vehicle
and industrial emissions on the variation of particle number concentration and its size
distribution during the same day.
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