Controlling magnetic anisotropy of a low symmetry metallic film by dynamical compressive and shear strain

Dynamical strain generated upon excitation of a metallic film by a femtosecond laser pulse may become a versatile tool enabling control of magnetic state of thin films and nanostructures via inverse magnetostriction on a picosecond time scale. Here we explore two alternative approaches to manipulate magnetocrystalline anisotropy and excite magnetization precession in a low-symmetry film of a magnetic metallic alloy galfenol (Fe,Ga) either by injecting picosecond strain pulse into it from a substrate or by generating dynamical strain of complex temporal profile in the film directly. In the former case we realize purely acoustic ultrafast control of magnetization by strain pulses. In the latter case optically-generated strain emerged abruptly in the film modifies its magnetoscrystalline anisotropy, competing with heat-induced change of anisotropy parameters. We demonstrate that the optically-generated strain remains efficient under conditions, when the heat-induced changes of anisotropy parameters do not trigger the precession anymore. We emphasize that the control of magnetic anisotropy in both approaches relies on mixed, compressive and shear, character of the dynamical strain, which emerges due to low-symmetry of the metallic film under study.