Artificial Carbon Graphdiyne: Status and Challenges in Nonlinear Photonic and Optoelectronic Applications.

The creative integration of sp-hybridized carbon atoms into artificial carbon graphdiyne has led to graphdiyne with superior properties in terms of uniformly distributed pores, ambipolar carrier transport, natural bandgap, and broadband absorption. Consequently, graphdiyne, regarded as a promising carbon material, has garnered particular attention in light-matter interactions. Light-matter interactions play an important role in optical information technology and meet the increasing demand for various energy sources. Herein, the status and challenges in nonlinear photonic and optoelectronic applications of graphdiyne, which are still in the infancy stage, are summarized. Furthermore, the bottleneck and perspective of graphdiyne in these aspects are discussed. It is therefore anticipated that this review could promote the development of graphdiyne in photonic and optoelectronic fields.