Structural dynamics of rotaxanes studied by infrared photon echo spectroscopy
2007
The structural dynamics of a rotaxane is investigated using infrared photon echo peak shift spectroscopy on the N-H stretch vibrational mode. The results demonstrate non-Markovian character of the dynamics of this vibrational mode and an oscillatory component related to the presence of low-frequency modes that are anharmonically coupled to the N-H stretch mode.
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