Temporal trends of novel brominated flame retardants in mollusks from the Chinese Bohai Sea (2011-2018).

Abstract Novel brominated flame retardants (NBFRs) have emerged as an alternative to traditional brominated flame retardants (BFRs); however, they may pose risks to the environment and human health. To investigate the occurrence, temporal trends, and human exposure of seven typical NBFRs (∑7 NBFRs), seven species of mollusks (n = 329) were collected from coastal cities in the Chinese Bohai Sea area from 2011 to 2018. The ∑7 NBFRs ranged from 1.52 to 154 ng/g dry weight (dw) (mean: 14.9 ± 21.21 ng/g dw), higher than in other areas worldwide. Decabromodiphenylethane (DBDPE) was the main contaminant, contributing to 33% of the NBFRs. Temporal trends indicate that the DBDPE and 2,3-dibromopropyl-2,4,6-tribromophenyl ether (DPTE) concentrations in mollusks increased significantly (P