Giant linear magnetoelectric effect at the morphotropic phase boundary of epitaxial Sr 0.5 Ba 0.5 MnO 3 films
2021
First-principles calculations are conducted to compute linear magnetoelectric coupling coefficients in epitaxial (001) ${\mathrm{Sr}}_{0.5}{\mathrm{Ba}}_{0.5}{\mathrm{MnO}}_{3}$ films. A large enhancement of different linear magnetoelectric elements is found in a strained-induced morphotropic phase boundary region. Such enhancement is demonstrated to originate from the behavior of the dielectric susceptibility, thanks to a simple phenomenological model that is presently shown to be relevant and accurate. This work can thus provide a promising approach towards designing highly desired single-phase multiferroic with a colossal magnetoelectric conversion.
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