Crystal field and magnetism with Wannier functions: rare-earth doped aluminum garnets
2015
Abstract Using the recently developed method we calculated the crystal field parameters in yttrium and lutetium aluminum garnets doped with seven trivalent Kramers rare-earth ions. We then inserted calculated parameters into the atomic-like Hamiltonian taking into account the electron-electron, spin-orbit and Zeeman interactions and determined the multiplet splitting by the crystal field as well as magnetic ĝ tensors. We compared calculated results with available experimental data. Very good agreement with the spectroscopic data and qualitative agreement with experimental ĝ tensors was found.
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