Applying a Template of Expected Uncertainties to Updating 239Pu(n,f) Cross-section Covariances in the Neutron Data Standards Database

Abstract Templates of uncertainties expected in specific measurement types were recently developed. One aim of these templates is to help evaluators in identifying (1) missing or suspiciously low uncertainties and (2) missing correlations between uncertainties of the same and different experiments, when estimating covariances for experimental data employed in their evaluations. These templates also provide realistic estimates of standard deviations and correlations for a particular uncertainty source and measurement type that can be used by evaluators in situations where they are not supplied by the experimenters. This information allows for a more comprehensive uncertainty analysis across all measurements considered in an evaluation and, thus, more realistic evaluated covariances. Here, we extend a template that is applicable to uncertainties expected in neutron-induced fission, (n,f), cross-section measurements. It is applied to improving covariances of 239Pu(n,f) cross-section measurements in the database underlying the Neutron Data Standards evaluations. This particular example was chosen since this evaluation is primarily based on experimental information. Also, some uncertainties of individual 239Pu(n,f) cross-section experiments in this database were suspected to be underestimated. The evaluated uncertainties obtained after updating the covariances in the database by means of the template indeed do increase compared to their original values. Even more importantly, the evaluated mean values change noticeably. These modified cross sections impact application calculations significantly, as is demonstrated by employing them in simulations of the effective neutron multiplication factor for a few selected critical assemblies. However, this updated evaluated 239Pu(n,f) cross section should not be interpreted as the final one that should replace values of the current Neutron Data Standards project. Evaluations for the Neutron Data Standards of the 239Pu(n,f) cross section must be linked to many other observables included in the associated database, most notably to cross sections for 235U(n,f), but also to those for 10B(n,α), 6Li(n,t), 238U(n,f), and 238U(n,γ), because of included measurements of the 239Pu(n,f) cross section that appear as ratios to these reactions. Some of these other reactions are correlated to further observables in the database. Hence, updating uncertainties of data sets of any of these observables can potentially impact the 239Pu(n,f) cross section. Uncertainties for all measurements of these linked physical observables have to be updated before a comprehensive evaluation of the 239Pu(n,f) cross section and its corresponding uncertainties can be provided.