OH survey along sightlines of Galactic Observations of Terahertz C

We have obtained OH spectra of four transitions in the (2)Pi(3/2) ground state, at 1612, 1665, 1667, and 1720 MHz, toward 51 sightlines that were observed in the Herschel project Galactic Observations of Terahertz C+. The observations cover the longitude range of (32 degrees, 64 degrees) and (189 degrees, 207 degrees) in the northern Galactic plane. All of the diffuse OH emissions conform to the so-called "Sum Rule" of the four brightness temperatures, indicating optically thin emission conditions for OH from diffuse clouds in the Galactic plane. The column densities of the H I "halos" N(H-I) surrounding molecular clouds increase monotonically with OH column density, N(OH), until saturating when N(H-I)= 1.0 x 10(21) cm(-2) and N(OH) >= 4.5 x 10(15) cm(-2), indicating the presence of molecular gas that cannot be traced by H I. Such a linear correlation, albeit weak, is suggestive of H (I) halos' contribution to the UV shielding required for molecular formation. About 18% of OH clouds have no associated CO emission (CO-dark) at a sensitivity of 0.07 K, but are associated with C+ emission. A weak correlation exists between C+ intensity and OH column density for CO-dark molecular clouds. These results imply that OH seems to be a better tracer of molecular gas than CO in diffuse molecular regions.