Enantioselective vinylogous Mukaiyama aldol reaction of α-ketoesters under bifunctional organocatalysis
2021
A highly enantioselective vinylogous Mukaiyama aldol reaction to ketoesters catalysed by a hydrogen-bond-donor-based bifunctional organocatalyst is presented. The addition of silyloxy dienol ether gives rise to multifunctional chiral tertiary alcohols bearing a versatile α,β-unsaturated aldehyde with excellent enantiocontrol.
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